This is easy, my favorite S+G song is “The Boxer”…having minimal Art Garfunkel involvement is a major argument in it’s favour… 
They never recorded it, but they did sing it in concerts. I have an ancient copy of an audiotape of a 1966 or so concert at Tufts University, which includes a nice rendition of this song.
Ahhh, I see. 
Thanks.
Sound of Silence and Bridge Over Troubled Waters, with Kathy’s Song a close third.
But I still think that the entire GD forum should adopt as its credo the line from The Boxer that Labdad quoted!
Dangling Conversation on the Parsley, Sage, Rosemary and Thyme album.
I also like At the Zoo.
This thread has inspired me to go pop in a S&G CD. Thanks!
As to my favorites, I’ll go with Bridge Over Troubled Water(makes me tear up in spite of myself), and The Boxer.
Like 'em all but Scarborough Fair always comes to mind.
Baby Driver makes me happy.
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At the Zoo
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I am a Rock
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Homeward Bound
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Bridge Over Troubled Water (doesn’t seem to be mentioned too times so far)
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Mrs. Robinson (imho, it was good in '68, but better now. And it was nice that JoeD finally figured out, or someone explained to him what the song was about. It’s an old story, but kind of funny. And that’s no knock against DiMaggio, either)
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Hazy Shade of Winter
Sounds of Silence narrowly edges out The Boxer
with Scarborough Affair/Canticle and April, Come She Will closely behind.
While I happily acknowledge all the classics listed above, I have a certain fondness for A Simple Desultory Philippic (Or How I Was) and The Dangling Conversation.
Though, of course, For Emily, Whenever I May Find Her, with its almost haunting etherial feeling still gets to me every time.
Interestingly, they’re all from “Parsley, Sage, Rosemary and Thyme,” which the AMG calls “an
achievement akin to the Beatles’ Revolver or the Beach Boys’ Pet Sounds album,” and that’s high praise indeed.