The problem is that you are trying to change out parts that are essentially antiques.
However, never under-estimate the ability of your local bike shop to keep, what should be by all rights, essentially worthless garbage sitting around waiting for the day that someone like you needs those parts. I was amazed when one of the older mechanics at my shop whipped out an early 1960’s era Campaganolo bottom bracket that was just what was need for a customers problem.
Your best bet if you are committed to keeping this bike would be to replace the entire drivetrain with a matched set of index shifting components.
That said, you may not need to touch the front deraileur and/or the crankset. Index shifting for the front deraileur is overrated (I mean, come on, there are only 2, maybe three chainrings, you can probably live with standard shifting). You also won’t need to change out the cranks as long as the new chain seats properly on the chainrings (index shifting chains generally altered the WIDTH of the chain, but the length between links is typically the same, and because the front chainring is less sensitive to width differences than the cogset, you may be ok there).
Assuming you can ignore the crankset and front deraileur, you will need a rear deraileur, a matched rear shifter, new chain, and a new cogset (make sure its a cogset that is compatible with your hub, I don’t think the hoods ever had cassette type cogset). A sticky issue is that you may not be able to find an index cogset that fits on your existing rear wheel hub. Cogsets have gotten progressively larger over the years as they have gone from 5 speeds to now typically 8-10 gears. This has changed both the sizing of the wheel hubs, as well as the bicycle frames themselves. So to get it all to work you may need to either find older index shifting parts that fit better with your setup, or use a newer cogset that may also require you to use a new wheel axle (or possibly even a new hub- which means a complete new wheel) to accomodate the greater width. If that is the case, you probably will also need to get into bending your frame to accomodate the wider axle spacing. Luckily, your frame is steel and responds well to the small tweaks that will be needed. See here for more info:
So, as you can see, it’s not exactly a straightforward task, and there are lots of issues that can potentially cause a cascading series of other issues. By the time you are done, it may be more money and effort than it’s worth when compared to buying a new or used bike with index shifting. Trek made a number of steel frame bikes back in the 90’s that had index shifting. I picked up one of those for my wife a couple of years ago for $35 from Craigslist (originally was about a $400).