The visual origins of "Violence Princess Ai"?

…as some of you may know, occasionally mentions a “staff member” named Violence Princess Ai. In fact, in one of their product listings, they show an animated GIF of the “Princess” wearing cybernetic armor.

Now, my question is: From what source did villainsupply take the “screen shots” of that make up the GIF? It looks like it might be from a movie of some sort, although the face looks like it might have been added later in Photoshop.

Can…anyone help?